Overview of the results of research of radioactive contamination of the Kakhovka Reservoir, which were conducted after the accident at the Chernobyl NPP (1986-1921)

Volodymyr Каnivets
Ukrainian Hydrometeorological Institute
https://orcid.org/0009-0008-1672-5547

Grydorii Derkach
Ukrainian Hydrometeorological Institute
https://orcid.org/0009-0006-4266-9126

DOI: http://doi.org/10.15407/Meteorology2024.05.027

Keywords: reservoir, bottom sediments, suspended sediments, radioactive contamination, cesium-137, strontium-90, becquerel

Abstract

The available data on the state of radioactive contamination of water and bottom sediments of the Kakhovka Reservoir were analyzed in order to assess the possible deterioration of the quality of the environment based on the indicators of radioactive contamination in the zone of influence of the emergency discharge of water due to destruction of the Kakhovka NPP dam by the Russian military. Contamination of the Kakhovka Reservoir with 137Cs occurred mainly through the fallouts of this radionuclide with aerosols on the water surface in May 1986. A much smaller part of this radionuclide transported by water runoff directly from the headwaters of the Dnieper basin. Strontium-90 entered the reservoir exclusively by water pathway starting from October 1986. The steady trends of decreasing activity of both radionuclides in water has been observed since 1987. Approximately to 1996 137Cs activity concentrations had decreased to pre-accident level, 90Sr activity demonstrated a slow decrease and by 2022 remained slightly higher than pre-accidental level. The average levels of contamination of the Kakhovka reservoir bottom with 137Cs and 90Sr turned out to be the lowest compared to the other reservoirs of the Dnieper cascade. It was shown that in 1994 137Cs activity levels were 0.06 Ci/km2(2,2 kBq/m2) on 80% of the bottom surface (submerged former floodplain of the Dnieper) and were lower than on the territory adjacent to the reservoir. In the areas of silt accumulation (former channel of the Dnieper) 137Cs activity was on average three times higher. Balance calculations based on the data of radiation monitoring of water showed that the amount of 137Cs activity in the bottom sediments in the period 1987-2022 halved due to natural radioactive decay, the amount of 90Sr activity decreased by approximately 20%, since activity losses due to natural radioactive decay were partially compensated by the constant supply of this radionuclide with water runoff from the contaminated part of the catchment. After a catastrophic water leak from the reservoir, the Dnieper floodplain had exposed. According to the calculations, the average density of soil contamination of the ехposed areas with 137Cs does not exceed 0.03 Ci/km2 (1,1 kBq/m2), with 90Sr – less than 0.1 Ci/km2 (3,7 kBq/m2). Silt deposits of the former Dnieper channel, which had an increased level of 137Cs contamination, were re-suspended, probably, and carried out into the Dnipro-Bug estuary and further into the Black Sea. However, according to our assumptions, this should not have a negative effect on the radioecological state of the sea, because the 137Cs activity concentrations in the water of north-western part of the Black Sea were always 20-30 times higher than in the Dnieper water.

References

1. Bochkov, L, Vakulovsky, S, Nikitin, A, Tertyshnik, E, Chumichev, V (1983). About the content of cesium-137 in surface waters of land. Meteorology and Hydrology, 8, 79–83. [In russian]

2. Bronnikov, V.K., Verkhovetsky, V.K., Nazipov, R.M., Barbashev, S.V. et al. (1994). Zaporozhskaya NPP and Environment. Kharkov. [In russian]

3. Gedeonov, L, Gritchenko, Z, Ivanova, L, Orlova, T, Tishkov, V, Toporkov, V, Prokopenko, V. (1993). Radionuclides of strontium and cesium in the water of the lower Danube in 1985–1990. Atomic Energy, 74(1), 58-63. [In russian]

4. IAEA (2006). Radiological Conditions in the Dnieper River Basin. IAEA RAR Series, Vienna.

5. Israel, Yu.A., Vakulovsky, S.M., Vetrov, V.A., Petrov, V.I., Rovinsky, F.Ya., Stukin, E.D. (1990). Chernobyl: radioactive contamination of natural environments. Leningrad, 296. [In russian]

6. Kanivets, V.V. (1996). Analysis of the main tendencies in the development of the radiation situation in the Dnieper water system after the Chernobyl accident. Bulletin of Agrarian Science, 4, 39-48. [In russian]

7. Kanivets, V.V., Derkach, G.A., Lutsenko, S.I. (2005). The state of radioactive contamination of river and sea waters of Ukraine two decades after the Chernobyl accident // Proceedings of the international. conf. “Radioactivity after nuclear explosions and accidents”, (Moscow, December 5-6, 2005). [In russian]

8. Kanivets, V., Laptev, G., Konoplev, A., Lisovyi, H., Derkach, G., Voitsekhovych, O. (2020). Dynamics of Radionuclides in the Chernobyl Cooling Pond. In: Konoplev, A., Kato, K., Kalmykov, S. (Eds). Behavior of Radionuclides in the Environment II: Chernobyl. Tokyo: Springer, 349–405. (https://doi.org/10.1007/978-981-15-3568-0_8)

9. Kanivets, V.V., Voitsekhovitch, O.V., Simov, V.G., Golubeva, Z.A. (1999). The post-Chernobyl budget of 137Cs and 90Sr in the Black Sea. Journal of Environmental Radioactivity, 43, 121-135.

10. Kanivets, V.V., Voitsekhovich, O.V., Khrystyuk, B.F., (1998). Riverine Transport of 137Cs and 90Sr into the Black Sea After Chernobyl Accident (Data Analysis and Methodological Aspects of Monitoring). Proc. of Inter. Sympos. on Marine Pollut. (Monaco, 5-9 October 1998), 44-51.

11. Kondratiev, N.E., Popov, I.V., Snischenko, B.F. (1982). Fundamentals of the hydromorphological theory of the channel process. Leningrad. [In russian]

12. Kulebakina, L.G. & Polikarpov, G.G. (1991). Radioecological Monitoring of the Black Sea Basin Following the Chernobyl NPS Accident. Proc. of Seminar on Comparative Assessment of the Environmental Impact of Radionuclides Released during Three Major Nuclear Accidents: Kyshtym, Windscale, Chernobyl. Luxembourg, 1-5 Oct. 1990, Luxembourg, Report EUR 13574, II, 607-648.

13. Kuzmenko, M.I., Volkova, E.N., Klenus, V.G., Novikov, B.I., Pan’kov, I.V., Kaglyan, A.E., Matvienko, L.P., Shirokaya, Z.O. (1992). Radioactive contamination of the Dnieper and its reservoirs and some hydroecological measures after the Chernobyl accident. Hydrobioljgical Journal, 28 (6): 86-94. [In russian]

14. Makhonko, K.P. (1987). Radioactive contamination of the territory of the USSR in 1986 (Yearbook) / edited by K.P. Makhonko, Obninsk.134. [In russian]

15. Novikov, B.I., Timchenko, V.M. (1992). Hydrological conditions for the migration of radionuclides along the cascade of Dnieper reservoirs. Water Resources, 1, 95-102. [In russian]

16. Polikarpov, G.G., Kulebakina, L.G., Timoshchuk, V.T., and Stokozov, N.A. (1991). Sr-90 and Cs-137 in Surface Waters of the Dnieper River, the Black Sea and the Aegen Sea in 1987 and 1988. Journal of Environmental Radioactivity, 13, 25-38.

17. Romanenko, V.D., Kuzmenko, M.I., Yevtushenko, M.Yu. et al. (1992). Radioactive and chemical contamination of the Dnieper and its reservoirs after the accident at the Chernobyl nuclear power plant. Kiev.

18. Sansone, U., Belli, M., Kanivets, V.V., Voitsekovitch, O.V. (1996). 137Cs and 90Sr in water and suspended particulate matter of the Dnieper River-Reservoirs System (Ukraine). Science of the Total Environment, 186 (3), 257-271.

19. Voitsekhovich, O.V., Kanivets V.V., Laptev G.V. (1997). Current state of radioactive contamination of water bodies in the zone affected by the accident // In the book: Radiogeoecology of water systems affected to contamination as a result of the Chernobyl accident. Kyiv, Chernobylinterinform, 60-96. [In russian]

20. Voitsekhovych, O., Kanivets, V., Simov, V., Fetisov, L. et al. (1996). Experimental Studies of the Radionuclide Flux from Rivers and Radionuclide-Sediment Interaction in the Black Sea. Final report under IAEA research contract No. 7330/R2/RB, UHMI, Kyiv.

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